1 Hey Schoolgirl / Black Slacks
2 That Silver Haired Daddy of Mine
3 The Sound of Silence
4 Star Carol
5 Comfort and Joy
6 The Sound of Silence (Acoustic Version)
7 Bye Bye Love (Live at Memorial Auditorium, Burlington, VT - October 1968)
8 A Most Peculiar Man (Live at Memorial Auditorium, Burlington, VT - October 1968)
9 The 59th Street Bridge Song (Feelin' Groovy)
10 Flowers Never Bend Wth the Rainfall
11 Red Rubber Ball (Live at Lincoln Center, New York City, NY - January 1967)
12 Red Rubber Ball
13 Blessed (Live at Lincoln Center, New York City, NY - January 1967)
14 A Church Is Burning (Live at Lincoln Center, New York City, NY - January 1967)
15 Save the Live of My Child
16 Old Friend/ Bookends
17 The Boxer (El Boxeador)
18 Program Open: America
19 We've Got a Groovy Thing Going On
20 Bleecker Street (Demo)
21 Overs (Live)
22 A Most Peculiar Man (Live)
23 So Long, Frank Lloyd Wright
24 Song for the Asking
25 The Dangling Conversation
26 Blues Run the Game
27 Hey Schoolgirl / Black Slacks - Live at Carnegie Hall, New York, NY - November 1969
28 That Silver Haired Daddy of Mine - Live at Carnegie Hall, New York, NY - November 1969
29 Mrs. Robinson - From "The Graduate" Soundtrack
30 Anji - Live at Lincoln Center, New York City, NY - January 1967
31 You Don't Know Where Your Interest Lies - Single B-Side - 1968
32 Bleecker Street - Demo - 1964
33 Blues Run the Game - Studio Outtake - 1965
34 The Sound of Silence - single version
35 Program Open: America